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Being a typical member of the lanthanide series, samarium usually assumes the oxidation state 3.

Compounds of samarium(II) are also known, most notably the monoxide Sm O, monochalcogenides Sm S, Sm Se and Sm Te, as well as samarium(II) iodide.

Mark Enderby reports on two (inactive) steam survivors in Yerevan (1st September 2008).